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Kenneth Haas

Synthesize acyl chloride from aldehyde

Allistar Evans  Follow

There are many ways to affect the transformation, as you have realised, and many of which Loong has detailed below in his post.

This answer gives one method which I would be confident of working practically, in the lab, using common reagents. A full search of Reaxys of SciFinder would reveal conditions/methods more suitable for a specific aldehyde.

A Pinnick oxidation will convert an aldehyde into its corresponding carboxylic acid, which may then be treated with a reagent such as oxalyl chloride to give the desired acyl chloride.

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Chr?s Odey  Follow

In some cases, the direct reaction with chlorine is possible:

2-chlorobenzaldehyde and dichlorine to 2-chlorobenzoyl chloride
Clarke, H. T.; Taylor, E. R. o-Chlorobenzoyl chloride. Org. Synth. 1929, Vol. 9, 34; 1941, Coll. Vol. 1, 155.

 

In other reactions, radical chlorinating agents are used:

aldehyde and tert-butyl hypochlorite to acyl chloride
Ginsburg, D. The Action of t-Butyl Hypochlorite on Organic Compounds. II. Aromatic Aldehydes. J. Am. Chem. Soc. 1951, 73 (2), 702–704.

 

aldehyde and N-chlorosuccinimide to acyl chloride
Hebbelynck, M. F.; Martin, R. H. Bull. Soc. Chim. Belg. 1951, 60, 54.

 

aldehyde and sulfuryl chloride to acyl chloride
Arai, M. Bull. Chem. Soc. Jpn. 1962, 35, 1272; 1964, 37, 1280; 1965, 38, 252.

 

aldehyde and sulfuryl chloride to acyl chloride
Winstein, S.; Seubold, F. H. Jr. Free radical reactions of aldehydes. J. Am. Chem. Soc. 1947, 69 (11), 2916–2917.

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